Born in the city of Luxembourg, Muller studies theology at the Grand Seminary of Metz, known for its Gallican orientation. In 1818, he is ordained a priest. This neo-humanist and Kantian adheres to the ideas of the constitutional church, which requires bishops and priests to swear an oath to the constitution. In 1813, Muller becomes a professor of Ancient Greek at the College of Luxembourg (the future Athenaeum), of which he becomes the director in 1821. Around the same time, he becomes a correspondent for the Journal de Luxembourg, a government newspaper run and printed by liberal Orangists, if not anti-clerical, and members of the Masonic lodge. In the 1840s, Muller is part of the Josephite clergy that Laurent despises.
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